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A key challenge in the characterization of ferroelectric domain walls is the determination of their structure and dynamics from the combination of high-resolution imaging and various physical properties. High-resolution scanning probe microscopy provides a direct technique for probing domain wall structure.
In the last decade, new high-resolution imaging tools have enabled direct imaging of the domain walls at the atomic resolution. The physical mechanisms of ferroelectric domain walls and their dynamics are now being investigated in the context of domain walls of ferroelectric perovskites at the atomic scale. There has been growing interest in the mechanical properties of ferroelectric walls, including their elasticity15,16, elastic instabilities17, and their ability to accommodate defects18. The domain walls are inherently dynamic objects, as evidenced by the domain wall dynamics in bulk ferroelectrics19,20, and the wall dynamics in thin ferroelectric films21,22,23,24. The unusual magnetoelectric coupling in multiferroic walls25,26 has been known since the dawn of ferroelectricity.
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